Evaluation of the Engineering Design Study Testing of the Batch

7,29
MB Supercritical Water Oxidation Process to Treat NSCMP

208
stron Neutralents and CAIS Materiel

3399
ID Department of Defense

2002
rok

Table of Contents

1. Introduction 1

1.1 Objectives. 1

1.1.1 Treat NSCMP Neutralent Material. 2

1.1.2 Treat CAIS Materiel 2

1.1.3 Fate of Heteroatoms and Material Balance Closure .. 2

1.1.4 Evaluate the Practicality for NSCMP 3

1.1.5 Develop Full-scale Processing Concept 3

1.1.6 Develop Plan for Next Phase of Testing.. 4

1.2 Evaluation Criteria 4

1.2.1 Treat NSCMP Neutralent Material. 4

1.2.2 Treat CAIS Materiel 4

1.2.3 Fate of Heteroatoms and Material Balance Closure .. 5

1.2.4 Evaluate the Practicality for NSCMP 5

1.2.5 Develop Full-scale Processing Concept 5

1.2.6 Develop Plan for Next Phase of Testing.. 6

2. Background 7

2.1 Technology Evaluation and Development for NSCMP. 7

2.2 Supercritical Water Oxidation. 8

3. System Description.. 10

4. Test Approach. 14

4.1 Test Matrix. 14

4.1.1 Workup Testing.. 14

4.1.2 Performance Testing 15

4.2 Feeds Tested.. 15

4.2.1 Neutralent Materials. 15

4.2.2 CAIS Materiels .. 15

4.3 Test Procedure – Liquid Neutralent .. 16

4.4 Test Procedure – CAIS. 19

5. Test Results & Discussion – Liquid Neutralents .. 20

5.1 Workup Testing 20

5.2 Performance Testing.. 25

5.3 Operability. 26

5.3.1 System Operation.. 26

5.3.2 Graylockä seals. 27

5.3.3 External heaters.. 27

5.3.4 External valving . 27

5.3.5 Instrumentation.. 27

5.3.6 Control and Data Acquisition. 28

5.4 Feed Analysis 28

5.4.1 Simulant analysis .. 28

5.4.2 Reactor Content Analysis.. 29

5.5 Residual characteristics 31

5.5.1 Gases.. 31

5.5.2 Liquid Residuals 36

5.5.3 Solids.. 39

5.6 Material Balance . 39

5.6.1 Destruction Efficiency 39

6. Test Results & Discussion – CAIS.. 41

6.1 Performance .. 41

7. Applicability to NSCMP 45

7.1 Batch-SCWO Processing Concepts .. 45

7.2 Phase 2 - Pilot Unit. 46

7.2.1 Processing Vessel Size 47

7.2.2 System Throughput.. 48

7.2.3 Corrosion Management.. 48

7.2.4 Vessel Configuration 49

7.2.5 Process/Equipment Operating Characteristics 50

7.2.6 Reliability, Availability and Maintainability.. 50

7.2.7 System Safety.. 51

7.3 Phase 3 - Munition Processing Size .. 52

7.3.1 Processing Vessel Size 53

7.3.2 System Throughput.. 54

7.3.3 Interface with Existing Munition Recovery. 54

7.3.4 Vessel Configuration 54

7.3.5 Corrosion Management.. 54

7.3.6 Process/Equipment Operating Characteristics 54

7.3.7 Reliability, Availability and Maintainability.. 55

7.3.8 System Safety.. 56

8. Conclusions .. 57

9. Recommendations. 58

10. References.. 59

Appendix A – Simulated CAIS Vial Specification

Appendix B – Analytical Report prepared by Southwest Research Institute

Appendix C – Batch-SCWO Vessel Analysis Calculation